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Interfacial chemistry regulation by orbital hybridization for superior kinetics of hard carbon in an ester-based electrolyte

Lu Liu, Jianhua Zhu, Guohui Chen, Zhuosen Wang, Liu Wang, Chengkun Guo, Yunfeng Chao, Xinwei Cui, Caiyun Wang

2025Chemical Science7 citationsDOIOpen Access PDF

Abstract

) in the ester-based electrolyte. Even the practical full cell showed no capacity decay over 400 cycles at 2C. This work provides a simple and effective interfacial modification strategy, offering new insights into the advancement of hard carbon anodes for high-performance SIBs.

Topics & Concepts

ElectrolyteAnodeNucleationCarbon fibersChemistrySodiumKineticsIonDiffusionChemical engineeringPolymer chemistryMaterials scienceInorganic chemistryOrganic chemistryPhysical chemistryElectrodeThermodynamicsComposite materialPhysicsComposite numberEngineeringQuantum mechanicsAdvanced Battery Materials and TechnologiesAdvancements in Battery MaterialsIonic liquids properties and applications