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Enhancing Strain-Sensing Properties of the Conductive Hydrogel by Introducing PVDF-TrFE

Zhirui Hu, Jie Li, Xiaotong Wei, Chen Wang, Yang Cao, Zhiqiang Gao, Jing Han, Yingchun Li

2022ACS Applied Materials & Interfaces72 citationsDOI

Abstract

-trifluoroethylene) (PVDF-TrFE) as the piezoelectric filler. A one-pot thermoforming and solution exchange method was used to synthesize the CHACC/PEDOT: PSS/PVDF-TrFE hydrogel. The hydrogel-based strain sensor exhibits very high sensitivity (GF: 19.3), fast response (response time: 63.2 ms), and wide frequency range (response frequency: 5-25 Hz), while maintaining excellent mechanical properties (elongation at break up to 293%). It can be concluded that enhanced strain-sensing properties of the hydrogel are contributed to both greater change in the relative resistance under stress and wider response to dynamic and static stimulus by adding PVDF-TrFE. This has a broad application in monitoring human motion, detecting subtle movements, and identifying object contours and a hydrogel-based array sensor. This work provides an insight into the design of composite hydrogels based on piezoelectric and piezoresistive sensing with applications for wearable sensors.

Topics & Concepts

Materials sciencePiezoresistive effectSelf-healing hydrogelsPEDOT:PSSComposite numberPiezoelectricityElectrical conductorComposite materialGauge factorPolymerFabricationPolymer chemistryPathologyMedicineAlternative medicineAdvanced Sensor and Energy Harvesting MaterialsConducting polymers and applicationsDielectric materials and actuators
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