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Huygens-Fresnel Picture for High Harmonic Generation in Solids

Liang Li, Pengfei Lan, Xiaosong Zhu, Peixiang Lu

2021Physical Review Letters36 citationsDOI

Abstract

High harmonic generation (HHG) is usually described by the laser-induced recollision of particlelike electrons, which lies at the heart of attosecond physics and also inspires numerous attosecond spectroscopic methods. Here, we demonstrate that the wavelike behavior of electrons plays an important role in solid HHG. By taking an analogy to the Huygens-Fresnel principle, an electron wave perspective on solid HHG is proposed by using the wavelet stationary-phase method. From this perspective, we have explained the deviation between the cutoff law predicted by the particlelike recollision model and the numerical simulation of semiconductor Bloch equations. Moreover, the emission times of HHG can be well predicted with our method involving the wave property of electrons. However, in contrast, the prediction with the particlelike recollision model shows obvious deviations compared to the semiconductor Bloch equations simulation. The wavelike properties of the electron motion can also be revealed by the HHG in a two-color field.

Topics & Concepts

PhysicsElectronHigh harmonic generationHarmonicCutoffSemiconductorAttosecondOpticsWaveformExcitationAmplitudeAtomic physicsWaveletNonlinear opticsEquations of motionWave propagationQuantum mechanicsComputational physicsMotion (physics)Laser-Matter Interactions and ApplicationsLaser Material Processing TechniquesAdvanced Electron Microscopy Techniques and Applications
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