Litcius/Paper detail

Dynamics of the electrically induced insulator-to-metal transition in rare-earth nickelates

Javier del Valle, Rodolfo Rocco, Claribel Domínguez, Jennifer Fowlie, Stefano Gariglio, M. J. Rozenberg, Jean‐Marc Triscone

2021Physical review. B./Physical review. B35 citationsDOIOpen Access PDF

Abstract

Rare-earth nickelates feature an insulator-to-metal transition (IMT) that can be electrically triggered. We study the dynamics of this electrically induced transition by comparing the time-dependent transport properties of two distinct members of the ${Re\mathrm{NiO}}_{3}$ family: ${\mathrm{NdNiO}}_{3}$ and ${\mathrm{SmNiO}}_{3}$. We report stark differences in the nucleation and growth of the metallic phase, which evolve more rapidly for ${\mathrm{NdNiO}}_{3}$. With the aid of simulations, we identify the amplitude of the resistivity change across the IMT as the key parameter controlling the switching speed. Our results are in accordance with recent experiments in the ${\mathrm{VO}}_{x}$ family, contributing to a unified vision of the field-induced IMT dynamics across different families of correlated oxides.

Topics & Concepts

Condensed matter physicsNucleationMetal–insulator transitionNon-blocking I/OElectrical resistivity and conductivityMaterials sciencePhase transitionRare earthMetalInsulator (electricity)PhysicsChemistryOptoelectronicsMetallurgyThermodynamicsQuantum mechanicsCatalysisBiochemistryMagnetic and transport properties of perovskites and related materialsAdvanced Condensed Matter PhysicsTransition Metal Oxide Nanomaterials