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Key difference between transition state stabilization and ground state destabilization: increasing atomic charge densities before or during enzyme–substrate binding

Deliang Chen, Yibao Li, Xun Li, Xuechuan Hong, Xiaolin Fan, Tor Savidge

2022Chemical Science130 citationsDOIOpen Access PDF

Abstract

and the mechanism of enhancing atomic charge densities. Our findings may help resolve the debate between TS stabilization and GS destabilization and assist our understanding of catalysis and the design of artificial enzymes.

Topics & Concepts

Key (lock)Substrate (aquarium)Charge (physics)Ground stateTransition (genetics)Chemical physicsState (computer science)Transition metalChemistryAtomic physicsMaterials scienceNanotechnologyPhysicsComputer scienceBiochemistryQuantum mechanicsBiologyCatalysisEcologyGeneComputer securityAlgorithmEnzyme Structure and FunctionAmino Acid Enzymes and MetabolismProtein Structure and Dynamics
Key difference between transition state stabilization and ground state destabilization: increasing atomic charge densities before or during enzyme–substrate binding | Litcius