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Temperature and doping-tuned coordination environments around electroactive centers in Fe-doped α(β)-Ni(OH)<sub>2</sub> for excellent water splitting

Qinghe Cao, Mi Luo, Yutian Huang, Qi Liu, Xiaoxing Kong, Jinlong Lei, Zheng Jiang, Jiahai Wang

2020Sustainable Energy & Fuels33 citationsDOI

Abstract

β-Ni(OH)<sub>2</sub> on Ni foam can be synthesized using a hydrothermal method. The addition of Fe<sup>3+</sup> during synthesis produced Fe-doped α-Ni(OH)<sub>2</sub> at 120 °C and Fe-doped β-Ni(OH)<sub>2</sub> at 240 °C. The HER and OER activity of these materials were investigated through both experiment and DFT.

Topics & Concepts

DopingHydrothermal circulationMaterials scienceWater splittingNickelHydrothermal synthesisInorganic chemistryPhysical chemistryAnalytical Chemistry (journal)Chemical engineeringChemistryMetallurgyOptoelectronicsCatalysisOrganic chemistryPhotocatalysisEngineeringElectrocatalysts for Energy ConversionAdvanced battery technologies researchCopper-based nanomaterials and applications
Temperature and doping-tuned coordination environments around electroactive centers in Fe-doped α(β)-Ni(OH)<sub>2</sub> for excellent water splitting | Litcius