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A Pillar[5]arene Conjugated Polymer for Removal of Low-Molecular-Weight Organic Acids, Amines, and Alcohols from Water

Zhuo Wang, Tao Chen, Guo Wang, Wei‐Bo Hu, Yahu A. Liu, Hui Yang, Ke Wen

2020ACS Applied Polymer Materials19 citationsDOI

Abstract

We have fabricated a pillar[5]arene-based conjugated polymer, pillar[4]arene[1]terephthalic acid-derivatized poly-p-phenylene pillar[4]arene[1]terephthamide (P[5]-PPTA), which demonstrated exceptional adsorption capability toward low-molecular-weight alkylamines, alcohols, and carboxylic acids in water. In addition, P[5]-PPTA could be thermally reactivated and reused at least five times without obvious decrease of adsorption capability. A mechanistic study indicated that the absorption results from the host–guest interaction between the pillar[5]arene rings in P[5]-PPTA and the low-molecular-weight short-chain alkyl derivatives.

Topics & Concepts

PillarAlkylPolymer chemistryAdsorptionConjugated systemChemistryPolymerTerephthalic acidOrganic chemistryPhenylenePolyesterEngineeringStructural engineeringSupramolecular Chemistry and ComplexesSupramolecular Self-Assembly in MaterialsLuminescence and Fluorescent Materials