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Bifurcated Halogen Bonding Involving Two Rhodium(I) Centers as an Integrated σ-Hole Acceptor

Anastasiya A. Eliseeva, Daniil M. Ivanov, Anton V. Rozhkov, Ivan V. Ananyev, Antonio Frontera, Vadim Yu. Kukushkin

2021JACS Au62 citationsDOIOpen Access PDF

Abstract

-orbitals of two positively charged rhodium(I) centers provide sufficient nucleophilicity to form a three-center halogen bond (XB) with the σ-hole donors. The two metal centers function as an integrated XB acceptor, providing assembly via a metal-involving XB.

Topics & Concepts

RhodiumHalogenAcceptorHalogen bondMaterials scienceChemistryCatalysisPhysicsOrganic chemistryCondensed matter physicsAlkylCrystallography and molecular interactionsOrganic and Molecular Conductors ResearchOrganic Chemistry Cycloaddition Reactions