Determination of the Néel vector in rutile altermagnets through x-ray magnetic circular dichroism: The case of <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:msub> <mml:mi>MnF</mml:mi> <mml:mn>2</mml:mn> </mml:msub> </mml:math>
Atsushi Hariki, T. Okauchi, Y. Takahashi, J. Kuneš
Abstract
We present a numerical simulation of x-ray magnetic circular dichroism (XMCD) at the ${L}_{2,3}$ edge of Mn in a representative rutile altermagnet ${\mathrm{MnF}}_{2}$ using a combination of density functional theory plus exact diagonalization of the atomic model. We explore how the dichroic spectra vary with the orientation of the light propagation vector and the N\'eel vector. An exact relationship between the XMCD spectra for different orientations of the N\'eel vector, valid in the absence of the valence spin-orbit coupling and core-valence multipole interaction, is derived and its approximate validity for the full Hamiltonian verified by numerical calculation. This relationship allows one to determine the in-plane orientation of the N\'eel vector using the XMCD spectra alone.