Litcius/Paper detail

Surface plasmon resonance sensing with thin films of palladium and platinum – quantitative and real-time analysis

John Andersson, Justas Svirelis, Gustav Ferrand‐Drake del Castillo, Takumi Sannomiya, Andreas Dahlin

2022Physical Chemistry Chemical Physics22 citationsDOIOpen Access PDF

Abstract

). Overall, the Pd sensors behave quite similarly to 50 nm gold in terms of sensitivity and field extension, although the noise level in real-time measurements is ∼5 times higher. The Pt sensors exhibit a longer extension of the evanescent field and ∼10 times higher noise compared to gold. Yet, formation of organic layers a few nm in thickness can still be monitored in real-time. As a model system, we use thiolated poly(ethylene glycol) to make Pd and Pt protein repelling. Our findings show how SPR can be used for studying chemical modifications of two metals that are important in several contexts, for instance within heterogeneous catalysis. We emphasize the advantages of simple sample preparation and accurate quantitative analysis in the planar geometry by Fresnel models.

Topics & Concepts

Surface plasmon resonancePalladiumPlanarPlatinumSurface plasmonAdsorptionMaterials scienceResonance (particle physics)PlasmonSurface (topology)Thin filmAnalytical Chemistry (journal)Localized surface plasmonOptoelectronicsNanotechnologyChemistryPhysical chemistryNanoparticleOrganic chemistryAtomic physicsPhysicsComputer scienceCatalysisMathematicsGeometryComputer graphics (images)Plasmonic and Surface Plasmon ResearchGold and Silver Nanoparticles Synthesis and ApplicationsOptical Coatings and Gratings