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Spodium Bonds: Noncovalent Interactions Involving Group 12 Elements

Antonio Bauzá, Ibón Alkorta, José Elguero, Tiddo J. Mooibroek, Antonio Frontera

2020Angewandte Chemie International Edition219 citationsDOIOpen Access PDF

Abstract

The term spodium (Sp) bond is proposed to refer to a net attractive interaction between any element of Group 12 and electron-rich atoms (Lewis bases or anions). These noncovalent interactions are markedly different from coordination bonds (antibonding Sp-ligand orbital involved). Evidence is provided for the existence of this interaction by calculations at the RI-MP2/aug-cc-pVTZ level of theory, atoms-in-molecules, and natural bond orbital analyses and by examining solid-state structures in the Cambridge Structure Database.

Topics & Concepts

Antibonding molecular orbitalNon-covalent interactionsChemistryGroup (periodic table)Natural bond orbitalLigand (biochemistry)Non-bonding orbitalCrystallographyMoleculeComputational chemistryChemical physicsMolecular orbitalElectronAtomic orbitalPhysicsDensity functional theoryQuantum mechanicsHydrogen bondOrganic chemistryReceptorBiochemistryCrystallography and molecular interactionsMetal-Organic Frameworks: Synthesis and ApplicationsCrystal structures of chemical compounds
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