Litcius/Paper detail

Low-Scaling Algorithms for <i>GW</i> and Constrained Random Phase Approximation Using Symmetry-Adapted Interpolative Separable Density Fitting

Chia-Nan Yeh, Miguel A. Morales

2024Journal of Chemical Theory and Computation21 citationsDOI

Abstract

We present low-scaling algorithms for GW and constrained random phase approximation based on a symmetry-adapted interpolative separable density fitting (ISDF) procedure that incorporates the space-group symmetries of crystalline systems. The resulting formulations scale cubically, with respect to system size, and linearly with the number of k -points, regardless of the choice of single-particle basis and whether a quasiparticle approximation is employed. We validate these methods through comparisons with published literature and demonstrate their efficiency in treating large-scale systems through the construction of downfolded many-body Hamiltonians for carbon dimer defects embedded in hexagonal boron nitride supercells. Our work highlights the efficiency and general applicability of ISDF in the context of large-scale many-body calculations with k -point sampling beyond density functional theory.

Topics & Concepts

ScalingRandom phase approximationSymmetry (geometry)Separable spaceContext (archaeology)Homogeneous spaceAlgorithmStatistical physicsQuasiparticleMathematicsPhysicsComputer scienceQuantum mechanicsMathematical analysisGeometryPaleontologySuperconductivityBiologyMachine Learning in Materials ScienceAdvanced Chemical Physics StudiesSurface Chemistry and Catalysis