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Single-molecule magnets within polyoxometalate-based frameworks

Malihe Babaei Zarch, Masoud Mirzaei, Maryam Bazargan, Sandeep K. Gupta, Franc Meyer, Joel T. Mague

2021Dalton Transactions40 citationsDOIOpen Access PDF

Abstract

, different void shapes, and the existence of dinuclear Tb(III) units only in 2. Frameworks 1 and 2 were further characterized by dc and ac magnetic measurements and both exhibit slow relaxation of magnetization at low temperatures under an applied dc field. Their single-molecule magnet (SMM) properties are investigated, where weak field-induced SMM behaviour is observed at low temperatures in dynamic magnetic studies.

Topics & Concepts

PolyoxometalateLanthanideCationic polymerizationMagnetizationSingle-molecule magnetThermogravimetric analysisMaterials scienceCrystallographyMoleculeInfrared spectroscopyChemistryIonMagnetic fieldPolymer chemistryOrganic chemistryPhysicsQuantum mechanicsCatalysisMagnetism in coordination complexesMetal-Organic Frameworks: Synthesis and ApplicationsPolyoxometalates: Synthesis and Applications