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Experimental investigation of the mechanism of supercritical CO2 interaction with tight sandstone

Huan Peng, Jian Yang, Junliang Peng, Junhong Pu, Qiang Liu, Jun Su, Jin Liu

2022Frontiers in Energy Research15 citationsDOIOpen Access PDF

Abstract

One of the important technologies for combating global climate change is CCUS (Carbon Capture, Utilization, and Storage), which aims to address the issue of “greenhouse effect” generated by a significant amount of greenhouse gas emissions. Supercritical CO 2 , a new type of anhydrous fracturing fluid with broad application prospects in low-pressure tight sandstone gas reservoirs, has several advantages over traditional water-based fracturing fluids, including quick flowback, minimal damage to the reservoir, and the ability to realize in-situ storage of greenhouse gases. The tight sandstone cores from the Jinqiu Gas field in the Sichuan Basin were used in an experimental investigation on the interaction mechanism between supercritical CO 2 and tight sandstone to examine the viability of supercritical CO 2 fracturing with tight sandstone, and analysis of the samples’ post-reaction samples’ mineral composition, microstructure, mass change, and total salinity change. The interaction of tight sandstone with supercritical CO 2 results in an increase in quartz content, a decrease in clay mineral content, the formation of new minerals, and partial mineral dissolution on the surface of the sample. Since the degree of mineral dissolution of sandstone samples increases with time, CO 2 can be stored in tight sandstone as carbonate minerals. This study evaluates how supercritical CO 2 interacts with tight sandstone and can offer a solid theoretical foundation and experimental evidence in favor of CO 2 in-situ storage in tight sandstone gas reservoir.

Topics & Concepts

Supercritical fluidDissolutionCarbon sequestrationCarbonateGeologyGreenhouse gasMineralogyCarbon capture and storage (timeline)Carbon dioxideClay mineralsHydraulic fracturingTight gasGeochemical modelingPetroleum engineeringChemical engineeringMaterials scienceChemistryClimate changeOceanographyMetallurgyOrganic chemistryEngineeringCO2 Sequestration and Geologic InteractionsHydraulic Fracturing and Reservoir AnalysisHydrocarbon exploration and reservoir analysis
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