Litcius/Paper detail

Direct Electro Plasmonic and Optic Modulation via a Nanoscopic Electron Reservoir

Wancong Li, Qiang Zhou, Pu Zhang, Xuewen Chen

2022Physical Review Letters11 citationsDOI

Abstract

Direct electrical tuning of localized plasmons at optical frequencies boasts the fascinating prospects of being ultrafast and energy efficient and having an ultrasmall footprint. However, the prospects are obscured by the grand challenge of effectively modulating the very large number of conduction electrons in three-dimensional metallic structures. Here we propose the concept of nanoscopic electron reservoir (NER) for direct electro plasmonic and electro-optic modulation. A NER is a few-to-ten-nanometer size metal feature on a metal host and supports a localized plasmon mode. We provide a general guideline to construct highly electrically susceptible NERs and theoretically demonstrate pronounced direct electrical tuning of the plasmon mode by exploiting the nonclassical effects of conduction electrons. Moreover, we show the electro-plasmonic tuning can be efficiently translated into modulation of optical scattering by utilizing the antenna effect of the metal host for the NER. Our work extends the landscape of electro plasmonic modulation and opens appealing new opportunities for quantum plasmonics.

Topics & Concepts

PlasmonElectronOptoelectronicsMaterials scienceModulation (music)Nanoscopic scalePhysicsNanotechnologyAcousticsQuantum mechanicsPlasmonic and Surface Plasmon ResearchGold and Silver Nanoparticles Synthesis and ApplicationsQuantum and electron transport phenomena