Correlation of the spin state and catalytic property of M–N<sub>4</sub>single-atom catalysts in oxygen reduction reactions
Wei Zhang, Jin-kong Pan, Yifan Yu, Xianjie Zhang, Jiahao Wang, Wen‐Xian Chen, Gui‐Lin Zhuang
Abstract
multi-angle electronic analysis. The spin states of catalysts play a crucial role in the activity and selectivity of ORRs mainly by manipulating the bond strength between OOH and catalysts. This will provide new insights for the rational design of ORR catalysts with magnetic metals.
Topics & Concepts
CatalysisChemistryOverpotentialDensity functional theorySelectivitySpin statesGrapheneDissociation (chemistry)ParamagnetismMetalPhotochemistryInorganic chemistryComputational chemistryPhysical chemistryMaterials scienceNanotechnologyOrganic chemistryElectrodePhysicsQuantum mechanicsElectrochemistryElectrocatalysts for Energy ConversionCatalytic Processes in Materials ScienceAdvanced battery technologies research