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Enhanced Photogating Gain in Scalable MoS<sub>2</sub> Plasmonic Photodetectors via Resonant Plasmonic Metasurfaces

Wei-Ren Syong, Jui‐Han Fu, Yu-Hsin Kuo, Yu-Cheng Chu, Mariam Hakami, Tzu-Yu Peng, Jason Lynch, Deep Jariwala, Vincent Tung, Yu‐Jung Lu

2024ACS Nano23 citationsDOI

Abstract

Absorption of photons in atomically thin materials has become a challenge in the realization of ultrathin, high-performance optoelectronics. While numerous schemes have been used to enhance absorption in 2D semiconductors, such enhanced device performance in scalable monolayer photodetectors remains unattained. Here, we demonstrate wafer-scale integration of monolayer single-crystal MoS 2 photodetectors with a nitride-based resonant plasmonic metasurface to achieve a high detectivity of 2.58 × 10 12 Jones with a record-low dark current of 8 pA and long-term stability over 40 days. Upon comparison with control devices, we observe an overall enhancement factor of >100; this can be attributed to the local strong EM field enhanced photogating effect by the resonant plasmonic metasurface. Considering the compatibility of 2D semiconductors and hafnium nitride with the Si CMOS process and their scalability across wafer sizes, our results facilitate the smooth incorporation of 2D semiconductor-based photodetectors into the fields of imaging, sensing, and optical communication applications.

Topics & Concepts

PhotodetectorOptoelectronicsPlasmonMaterials scienceSemiconductorMonolayerWaferNanotechnology2D Materials and ApplicationsPlasmonic and Surface Plasmon ResearchMetamaterials and Metasurfaces Applications
Enhanced Photogating Gain in Scalable MoS<sub>2</sub> Plasmonic Photodetectors via Resonant Plasmonic Metasurfaces | Litcius