Litcius/Paper detail

Decarboxylative Polyfluoroarylation of Alkylcarboxylic Acids

Xiang Sun, Tobias Ritter

2021Angewandte Chemie International Edition65 citationsDOIOpen Access PDF

Abstract

Polyfluoroarenes are useful building blocks in several areas such as drug discovery, materials, and crop protection. Herein, we report the first polyfluoroarylation of aliphatic carboxylic acids via photoredox decarboxylation. The method proceeds with broad substrate scope and high functional group tolerance. Moreover, small complex molecules such as natural products and drugs can be modified by late-stage modification.

Topics & Concepts

DecarboxylationScope (computer science)Substrate (aquarium)ChemistryCombinatorial chemistryFunctional groupSmall moleculeOrganic chemistryComputer scienceBiologyCatalysisBiochemistryEcologyPolymerProgramming languageFluorine in Organic ChemistryRadical Photochemical ReactionsSulfur-Based Synthesis Techniques