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Visualizing the atomic-scale origin of metallic behavior in Kondo insulators

Harris Pirie, Eric Mascot, C. E. Matt, Yu Liu, Pengcheng Chen, Mohammad Hamidian, Shanta Saha, Xiangfeng Wang, Johnpierre Paglione, G. M. Luke, David Goldhaber‐Gordon, Cyrus F. Hirjibehedin, J. C. Davis, Dirk K. Morr, Jennifer E. Hoffman

2023Science23 citationsDOIOpen Access PDF

Abstract

A Kondo lattice is often electrically insulating at low temperatures. However, several recent experiments have detected signatures of bulk metallicity within this Kondo insulating phase. In this study, we visualized the real-space charge landscape within a Kondo lattice with atomic resolution using a scanning tunneling microscope. We discovered nanometer-scale puddles of metallic conduction electrons centered around uranium-site substitutions in the heavy-fermion compound uranium ruthenium silicide (URu 2 Si 2 ) and around samarium-site defects in the topological Kondo insulator samarium hexaboride (SmB 6 ). These defects disturbed the Kondo screening cloud, leaving behind a fingerprint of the metallic parent state. Our results suggest that the three-dimensional quantum oscillations measured in SmB 6 arise from Kondo-lattice defects, although we cannot exclude other explanations. Our imaging technique could enable the development of atomic-scale charge sensors using heavy-fermion probes.

Topics & Concepts

Kondo insulatorKondo effectCondensed matter physicsMaterials sciencePhysicsElectronQuantum mechanicsRare-earth and actinide compoundsTopological Materials and PhenomenaAdvanced Materials Characterization Techniques
Visualizing the atomic-scale origin of metallic behavior in Kondo insulators | Litcius