Efficient and stable photocatalytic H<sub>2</sub> evolution by self-assembly of zirconium(<scp>iv</scp>) coordination with perylene diimide supramolecules under visible light irradiation
Haoran Ding, Zhiqiang Wang, Kangyi Kong, Shufan Feng, Lifeng Xu, Haonan Ye, Wenjun Wu, Xue‐Qing Gong, Jianli Hua
Abstract
Self-assembly of Zr<sup>IV</sup> coordination with PDI supramolecules can facilitate separation and transfer of charge carriers. The photocatalyst <bold>P-PMPDI-Zr</bold> (1 : 0.25) achieved a superior HER activity of 50.46 mmol g<sup>−1</sup> h<sup>−1</sup> with an AQY of 11.7% at 630 nm.
Topics & Concepts
DiimidePerylenePhotocatalysisVisible spectrumZirconiumSelf-assemblyPhotochemistryIrradiationCrystallographyMaterials sciencePhotosensitivityChemistryNanotechnologyInorganic chemistryCatalysisOrganic chemistryMoleculePhysicsOptoelectronicsNuclear physicsAdvanced Photocatalysis TechniquesElectrocatalysts for Energy ConversionMetal-Organic Frameworks: Synthesis and Applications