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Synthesis and characterisation of Ga- and In-doped CdS by solventless thermolysis of single source precursors

Suliman A. Alderhami, Ruben Ahumada‐Lazo, Mark A. Buckingham, David J. Binks, Paul O’Brien, David Collison, David J. Lewis

2023Dalton Transactions13 citationsDOIOpen Access PDF

Abstract

materials were examined by UV-Vis absorption and photoluminescence spectroscopies respectively. All materials were found to exhibit excitonic emission, corresponding to band gap energies between 2.7 and 2.9 eV and surface defect induced emission which is more prominent for Ga than for In doping. Additionally, moderate doping slows down charge carrier recombination by increasing the lifetimes of excitonic and surface state emissions, but particularly for the latter process.

Topics & Concepts

PhotoluminescenceDopingThermal decompositionExcitonMaterials scienceRecombinationPhase (matter)Charge carrierSpectroscopyDecompositionChemical engineeringPhotochemistryChemistryOptoelectronicsOrganic chemistryCondensed matter physicsEngineeringBiochemistryGeneQuantum mechanicsPhysicsQuantum Dots Synthesis And PropertiesChalcogenide Semiconductor Thin FilmsMolecular Junctions and Nanostructures
Synthesis and characterisation of Ga- and In-doped CdS by solventless thermolysis of single source precursors | Litcius