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Second gadolinium loading to Super-Kamiokande

K. Abe, C. Bronner, Y. Hayato, K. Hiraide, K. Hosokawa, K. Ieki, M. Ikeda, J. Kameda, Y. Kanemura, R. Kaneshima, Y. Kashiwagi, Y. Kataoka, S. Miki, S. Mine, M. Miura, S. Moriyama, Y. Nakano, M. Nakahata, S. Nakayama, Y. Noguchi, Kenta Sato, H. Sekiya, H. Shiba, K. Shimizu, M. Shiozawa, Y. Sonoda, Y. Suzuki, A. Takeda, Y. Takemoto, Hiroyuki Tanaka, T. Yano, S. Han, T. Kajita, K. Okumura, T. Tashiro, Tomoaki Tomiya, X. Wang, S. Yoshida, P. Fernández, L. Labarga, N. Ospina, Bryan Zaldívar, B. W. Pointon, E. Kearns, J. L. Raaf, L. Wan, T. Wester, J. Bian, N.J. Griskevich, M. B. Smy, H. W. Sobel, Volodymyr Takhistov, A. Yankelevich, J. Hill, M. C. Jang, S.H Lee, D.H Moon, R. G. Park, B. Bodur, K. Scholberg, C. W. Walter, A. Beauchêne, O. Drapier, A. Giampaolo, Th. A. Mueller, Andrew D. Santos, Pascal Paganini, B. Quilain, R. Rogly, T. Nakamura, J.S Jang, L. N. Machado, J. G. Learned, K. Choi, N. Iovine, S. Cao, L. H. V. Anthony, D. Martin, N. W. Prouse, M. Scott, Y. Uchida, V. Berardi, N. F. Calabria, M. G. Catanesi, E. Radicioni, A. Langella, G. De Rosa, G. Collazuol, F. Iacob, M. Mattiazzi, L. Ludovici, M. Gonin, Lorenzo Périssé, G. Pronost, C. Fujisawa, Y. Maekawa, Y. Nishimura, R. Okazaki, R. Akutsu, M. Friend

2024Nuclear Instruments and Methods in Physics Research Section A Accelerators Spectrometers Detectors and Associated Equipment19 citationsDOIOpen Access PDF

Abstract

The first loading of gadolinium (Gd) into Super-Kamiokande in 2020 was successful, and the neutron capture efficiency on Gd reached 50%. To further increase the Gd neutron capture efficiency to 75%, 26.1 tons of Gd2(SO4)3⋅8H2O was additionally loaded into Super-Kamiokande (SK) from May 31 to July 4, 2022. As the amount of loaded Gd2(SO4)3⋅8H2O was doubled compared to the first loading, the capacity of the powder dissolving system was doubled. We also developed new batches of gadolinium sulfate with even further reduced radioactive impurities. In addition, a more efficient screening method was devised and implemented to evaluate these new batches of Gd2(SO4)3⋅8H2O. Following the second loading, the Gd concentration in SK was measured to be 333.5±2.5 ppm via an Atomic Absorption Spectrometer (AAS). From the mean neutron capture time constant of neutrons from an Am/Be calibration source, the Gd concentration was independently measured to be 332.7 ± 6.8(sys.) ± 1.1(stat.) ppm, consistent with the AAS result. Furthermore, during the loading the Gd concentration was monitored continually using the capture time constant of each spallation neutron produced by cosmic-ray muons, and the final neutron capture efficiency was shown to become 1.5 times higher than that of the first loaded phase, as expected.

Topics & Concepts

GadoliniumNeutron captureRadiochemistryNeutronSuper-KamiokandeChemistryNeutron poisonAnalytical Chemistry (journal)Materials scienceNeutron temperatureNuclear physicsPhysicsChromatographyNeutrinoMetallurgySolar neutrinoNeutrino oscillationNuclear Physics and ApplicationsNuclear reactor physics and engineeringRadiation Detection and Scintillator Technologies
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