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Metamagnetic transition and anomalous Hall effect in Mn-based kagomé magnets <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mi>R</mml:mi><mml:msub><mml:mi mathvariant="normal">Mn</mml:mi><mml:mn>6</mml:mn></mml:msub><mml:msub><mml:mi mathvariant="normal">Ge</mml:mi><mml:mn>6</mml:mn></mml:msub><mml:mrow><mml:mo>(</mml:mo><mml:mi>R</mml:mi><mml:mo>=</mml:mo><mml:mi mathvariant="normal">Tb</mml:mi><mml:mtext>−</mml:mtext><mml:mi mathvariant="normal">Lu</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math>

Huibin Zhou, Mengyi Shi, Yuqing Huang, Wenlong Ma, Xitong Xu, Junfeng Wang, Shuang Jia

2023Physical Review Materials12 citationsDOI

Abstract

We investigate electrical transport and magnetic properties of the single-crystalline, Mn-based kagom\'e magnets $R{\mathrm{Mn}}_{6}{\mathrm{Ge}}_{6}$ ($R$=Tb-Lu). The compounds mostly feature a series of magnetic orderings of $R$ and Mn moments at different temperatures and metamagnetic transition (MMT) under an external magnetic field. We classify the MMT into three types, i.e., from skewed spiral to a structure containing decoupled $R$ and Mn moments, from antiferromagnetic to flat spiral Mn moments, and from flat spiral to a ferrimagnetic state of $R$ and Mn moments. The former two induce a small anomalous Hall effect (AHE), whereas the latter gives rise to a large one. We conclude that ferromagnetic ordered Mn moments in the kagom\'e lattice lead to a significant AHE, while other magnetic structures of $R$ and Mn moments do not. The AHE in ${\mathrm{TbMn}}_{6}{\mathrm{Ge}}_{6}$ generally has an intrinsic origin, while no clear sign of intrinsic AHE is found in other compounds.

Topics & Concepts

FerrimagnetismAntiferromagnetismCondensed matter physicsMaterials scienceFerromagnetismMagnetic momentPhysicsMagnetic fieldMagnetizationQuantum mechanicsTopological Materials and PhenomenaAdvanced Condensed Matter PhysicsPhysics of Superconductivity and Magnetism