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Synthesis and structural characterisation of solid titanium(<scp>iv</scp>) phosphate materials by means of X-ray absorption and NMR spectroscopy

Daniela Rusanova-Naydenova, Mylène Trublet, Wantana Klysubun, Chanakan Cholsuk, Dinu Iuga, R. Dupree, Oleg N. Antzutkin, Ingmar Persson

2022Dalton Transactions14 citationsDOIOpen Access PDF

Abstract

Ti NMR and Ti pre-edge XANES show evidence of two different titanium environments in LTP, one very similar to that observed in TiP1-H and a second more symmetric octahedral environment. Data are discussed in terms of induced acidic hydrolyses of titanium(IV) and phosphate counterpart during washings with hydrochloric acid and water. A straightforward relation between synthesis parameters/post synthetic treatment and structural re-arrangement in the materials is established.

Topics & Concepts

Extended X-ray absorption fine structureTitaniumXANESOctahedronChemistryCrystallographyPhosphateInorganic chemistryNuclear magnetic resonance spectroscopySpectroscopyAbsorption spectroscopyCrystal structureStereochemistryOrganic chemistryPhysicsQuantum mechanicsChemical Synthesis and CharacterizationRadioactive element chemistry and processingBone Tissue Engineering Materials
Synthesis and structural characterisation of solid titanium(<scp>iv</scp>) phosphate materials by means of X-ray absorption and NMR spectroscopy | Litcius