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Photoluminescence Anisotropy in Eutectic Crystals of Polynuclear Lanthanide Complexes and Silver Clusters

Feifan Wang, Yu-Chen Zhang, Teng Zhao, Pengfei Feng, Zhenda Lu, Shuang‐Quan Zang, Thomas C. W. Mak

2023Angewandte Chemie International Edition12 citationsDOI

Abstract

Anisotropy is an intrinsic property of crystalline materials. However, the photoluminescence anisotropy in eutectic crystals of organometallic complexes has remained unexplored. Herein, the eutectic of polynuclear lanthanide complexes and Ag clusters was prepared, and the crystal shows significant photoluminescence anisotropy. The polarization anisotropy of emission δ and degree of excitation polarization P are 2.62 and 0.53, respectively. The rare excitation polarization properties have been proved to be related to the regular arrangement of electric transition dipole moments of luminescent molecules in the crystal. Our design provides a reference for developing new photoluminescence anisotropy materials and expanding their applications.

Topics & Concepts

PhotoluminescenceAnisotropyMaterials scienceLuminescenceLanthanidePolarization (electrochemistry)Eutectic systemCrystallographyDipoleCrystal (programming language)ChemistryOptoelectronicsAlloyPhysical chemistryOpticsMetallurgyOrganic chemistryPhysicsIonProgramming languageComputer scienceNanocluster Synthesis and ApplicationsLanthanide and Transition Metal ComplexesMagnetism in coordination complexes
Photoluminescence Anisotropy in Eutectic Crystals of Polynuclear Lanthanide Complexes and Silver Clusters | Litcius