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Heterogeneous Interactions of Prevalent Indoor Oxygenated Organic Compounds on Hydroxylated SiO<sub>2</sub> Surfaces

Liubin Huang, Elianna S. Frank, Mona Shrestha, Saleh Riahi, Douglas J. Tobias, Vicki H. Grassian

2021Environmental Science & Technology14 citationsDOI

Abstract

surface is driven by π hydrogen bonding and O-H hydrogen bonding interactions, with O-H hydrogen bonding interactions being stronger. The results of kinetic measurements suggest that indoor surfaces play a significant role in the removal of these OOCs, especially under moderate and low air exchange. Additionally, indoor surfaces can also serve as a reservoir of OOCs due to their much slower desorption kinetics when compared to other indoor relevant organic compounds such as limonene. Overall, the results gleaned by experiment and theoretical simulations provide a molecular representation of the interaction of OOCs on indoor relevant surfaces as well as implications of these interactions for indoor air chemistry.

Topics & Concepts

ChemistryIndoor airAdsorptionDesorptionHydrogen bondEnvironmental chemistryIndoor air qualityChemical physicsComputational chemistryPhysical chemistryOrganic chemistryMoleculeEnvironmental scienceEnvironmental engineeringIndoor Air Quality and Microbial ExposureAdvanced Chemical Sensor TechnologiesOdor and Emission Control Technologies
Heterogeneous Interactions of Prevalent Indoor Oxygenated Organic Compounds on Hydroxylated SiO<sub>2</sub> Surfaces | Litcius