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Experimental and theoretical studies on NIR luminescence of titanate‐germanate glasses doped with Pr <sup>3+</sup> and Tm <sup>3+</sup> ions

Marta Kuwik, Karolina Kowalska, Joanna Pisarska, Wojciech A. Pisarski

2023Journal of the American Ceramic Society15 citationsDOI

Abstract

Abstract Near‐infrared (NIR) luminescence of Pr 3+ and Tm 3+ ions in titanate‐germanate glasses has been studied for laser and fiber amplifier applications. The effect of the molar ratio GeO 2 :TiO 2 (from 5:1 to 1:5) on spectroscopic properties of glass systems was studied by absorption, luminescence measurements, and theoretical calculations using the Judd–Ofelt theory. It was found that independent of the TiO 2 concentration, intense NIR emissions at 1.5 and 1.8 μm were observed for glasses doped with Pr 3+ and Tm 3+ ions, respectively. Moreover, several spectroscopic and NIR laser parameters for Pr 3+ and Tm 3+ ions, such as emission bandwidth, stimulated emission cross‐section, quantum efficiency, gain bandwidth, and figure of merit, were determined. The results were discussed in detail and compared to the different laser glasses. Systematic investigations indicate that Pr 3+ ‐doped system with GeO 2 :TiO 2 = 2:1 and Tm 3+ ‐doped glass with GeO 2 :TiO 2 = 1:2 present profit laser parameters and could be successfully applied to NIR lasers and broadband optical amplifiers.

Topics & Concepts

GermanateLuminescenceMaterials scienceIonLaserDopingAnalytical Chemistry (journal)TitanateFigure of meritOpticsOptoelectronicsChemistryCeramicPhysicsComposite materialOrganic chemistryChromatographyGlass properties and applicationsLuminescence Properties of Advanced MaterialsSolid State Laser Technologies