Litcius/Paper detail

A heterometallic [LnLn′Ln] lanthanide complex as a qubit with embedded quantum error correction

Emilio Macaluso, Marcos Rubín-Osanz, David Aguilà, Alessandro Chiesa, Leoní A. Barrios, Jesús I. Martínez, Pablo J. Alonso, Olivier Roubeau, Fernando Luis, Guillem Aromı́, Stefano Carretta

2020Chemical Science78 citationsDOIOpen Access PDF

Abstract

We show that a [Er-Ce-Er] molecular trinuclear coordination compound is a promising platform to implement the three-qubit quantum error correction code protecting against pure dephasing, the most important error in magnetic molecules. We characterize it by preparing the [Lu-Ce-Lu] and [Er-La-Er] analogues, which contain only one of the two types of qubit, and by combining magnetometry, low-temperature specific heat and electron paramagnetic resonance measurements on both the elementary constituents and the trimer. Using the resulting parameters, we demonstrate by numerical simulations that the proposed molecular device can efficiently suppress pure dephasing of the spin qubits.

Topics & Concepts

DephasingQubitElectron paramagnetic resonanceLanthanideQuantumSpin (aerodynamics)MagnetometerMoleculeChemistryExchange interactionTopology (electrical circuits)PhysicsQuantum mechanicsMathematicsFerromagnetismMagnetic fieldThermodynamicsIonCombinatoricsMagnetism in coordination complexesLanthanide and Transition Metal ComplexesQuantum and electron transport phenomena