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Interaction Effects between the Main Components of Protein-Rich Biomass during Microwave-Assisted Pyrolysis

Cheng Hou, Chenxi Zhou, Nan Li, Yuanbo Song, Xiaogang You, Jiang Zhao, Xuefei Zhou, Zheng Shen, Yalei Zhang

2024Environmental Science & Technology24 citationsDOI

Abstract

The interaction effects between the main components (proteins (P), carbohydrates (C), and lipids (L)) of protein-rich biomass during microwave-assisted pyrolysis were investigated in depth with an exploration of individual pyrolysis and copyrolysis (PC, PL, and CL) of model compounds. The average heating rate of P was higher than those of C and L, and the interactions in all copyrolysis groups reduced the max instant heating rate. The synergistic extent ( S ) of PC and PL for bio-oil yield was 16.78 and 18.24%, respectively, indicating that the interactions promoted the production of bio-oil. Besides, all of the copyrolysis groups exhibited a synergistic effect on biochar production ( S = 19.43–28.24%), while inhibiting the gas generation, with S ranging from −20.17 to −6.09%. Regarding the gaseous products, apart from H 2, P, C, and L primarily generated CO 2, CO, and CH 4, respectively. Regarding bio-oil composition, the interactions occurring within PC, PL, and CL exhibited a significantly synergistic effect ( S = 47.81–412.96%) on the formation of N -heterocyclics/amides, amides/nitriles, and acids/esters, respectively. Finally, the favorable applicability of the proposed interaction effects was verified with microalgae. This study offers valuable insights for understanding the microwave-assisted pyrolysis of protein-rich biomass, laying the groundwork for further research and process optimization.

Topics & Concepts

PyrolysisBiomass (ecology)ChemistryMicrowaveChemical engineeringOrganic chemistryBiologyEcologyComputer scienceEngineeringTelecommunicationsThermochemical Biomass Conversion ProcessesEnergy and Environment ImpactsCatalysis and Hydrodesulfurization Studies
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