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Evidence of Lifshitz Transition in the Thermoelectric Power of Ultrahigh-Mobility Bilayer Graphene

Aditya Jayaraman, Kimberly Hsieh, Bhaskar Ghawri, Phanibhusan S. Mahapatra, Kenji Watanabe, Takashi Taniguchi, Arindam Ghosh

2021Nano Letters23 citationsDOIOpen Access PDF

Abstract

Resolving low-energy features in the density of states (DOS) holds the key to understanding a wide variety of rich novel phenomena in graphene-based 2D heterostructures. The Lifshitz transition in bilayer graphene (BLG) arising from trigonal warping has been established theoretically and experimentally. Nevertheless, the experimental realization of its effects on transport properties has been challenging because of its relatively low energy scale (∼1 meV). In this work, we demonstrate that the thermoelectric power (TEP) can be used as an effective probe to investigate fine changes in the DOS of BLG. We observed additional entropy features in the vicinity of the charge neutrality point (CNP) in gapped BLG. This apparent violation of the Mott formula can be explained quantitatively by considering the effects of trigonal warping, thereby serving as possible evidence of a Lifshitz transition.

Topics & Concepts

Condensed matter physicsGrapheneSeebeck coefficientBilayer grapheneBilayerMaterials scienceThermoelectric effectNanotechnologyEngineering physicsPhysicsChemistryThermodynamicsMembraneBiochemistryGraphene research and applicationsThermal properties of materialsAdvanced Thermoelectric Materials and Devices
Evidence of Lifshitz Transition in the Thermoelectric Power of Ultrahigh-Mobility Bilayer Graphene | Litcius