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Electrochemically enabled cobalt catalyzed enantioselective C–H acyloxylation of aryl phosphamide with carboxylic acid

Xuying Xia, Changdi Zheng, Yunfei Hang, Jiyuan Guo, Tao Liu, Dingguo Song, Zhiwei Chen, Weihui Zhong, Fei Ling

2024Green Chemistry25 citationsDOI

Abstract

We described here the first example of cobalt-electro-catalyzed enantioselective C–H acyloxylation of arylphosphinamides with carboxylic acids to generate P-stereogenic scaffolds.

Topics & Concepts

Enantioselective synthesisCatalysisChemistryCobaltCarboxylic acidElectrochemistryArylOrganic chemistryCombinatorial chemistryElectrodePhysical chemistryAlkylAsymmetric Hydrogenation and CatalysisCatalytic C–H Functionalization MethodsChemical Reactions and Isotopes