Litcius/Paper detail

Free Carboxylic Acids: The Trend of Radical Decarboxylative Functionalization

Liubo Li, Yan Yao, Niankai Fu

2023European Journal of Organic Chemistry131 citationsDOI

Abstract

Abstract The exceptional versatility of carboxylic acids has been extensively exploited in organic synthesis across several decades. There has been a recent upsurge of radical decarboxylative transformations. The process can be initiated under mild conditions, and the resultant radicals have orthogonal reactivities to closed‐shell species, thus providing immense opportunities for streamlining novel reactions. The use of free carboxylic acids is the most desirable owing to its high atom and step economy. Aiming to demonstrate the attractiveness of the strategy and to inspire chemists to tackle existing challenges, this review outlines the recent advances on radical decarboxylative functionalization of free carboxylic acids.

Topics & Concepts

ChemistryRadicalSurface modificationAtom economyDecarboxylationOrganic chemistryCarboxylic acidCombinatorial chemistryCatalysisPhysical chemistryRadical Photochemical ReactionsCatalytic C–H Functionalization MethodsSulfur-Based Synthesis Techniques