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Delamination of Ti<sub>3</sub>C<sub>2</sub>T<sub><i>x</i></sub> Nanosheets with NaCl and KCl for Improved Environmental Stability of MXene Films

Mikhail Shekhirev, Yusuke Ogawa, Christopher E. Shuck, Mark Anayee, Takeshi Torita, Yury Gogotsi

2022ACS Applied Nano Materials55 citationsDOI

Abstract

Two-dimensional titanium carbide (Ti3C2Tx; MXene) is the most important member of the MXene family with attractive properties and applications in energy storage, electronics, medicine, and many others. A typical synthesis involves selective etching of a layered precursor (MAX phase), followed by intercalation with Li+ ions and delamination into individual flakes. Here, we demonstrate that, by adjusting the etching conditions, Ti3C2Tx MXene can be delaminated with Na+ and K+. Since residual delamination agents are still present on the MXene surface after the delamination process, this protocol allows one to avoid adverse effects of Li+ and to improve the environmental stability of the films.

Topics & Concepts

Delamination (geology)Titanium carbideMaterials scienceIntercalation (chemistry)Etching (microfabrication)CarbideX-ray photoelectron spectroscopyPhase (matter)Chemical engineeringNanotechnologyComposite materialInorganic chemistryChemistryLayer (electronics)PaleontologyTectonicsBiologyEngineeringSubductionOrganic chemistryMXene and MAX Phase Materials2D Materials and ApplicationsAdvanced Memory and Neural Computing
Delamination of Ti<sub>3</sub>C<sub>2</sub>T<sub><i>x</i></sub> Nanosheets with NaCl and KCl for Improved Environmental Stability of MXene Films | Litcius