Litcius/Paper detail

AIBN-Induced Remote Trifluoromethyl-Alkynylation of Thioalkynes

Zhimin Xiong, Fang Zhang, Yongqi Yu, Ze Tan, Gangguo Zhu

2020Organic Letters44 citationsDOI

Abstract

A novel α,α′-azobis(isobutyronitrile) (AIBN)-induced remote trifluoromethyl-alkynylation of thioalkynes with alkynyl triflones as both the trifluoromethyl and alkyne sources is described. Structurally diverse trifluoromethylated (Z)-enynes can be constructed with full control of regio-, stereo-, and site-selectivity, which serves as a highly selective method for the rapid construction of trifluoromethylated molecules.

Topics & Concepts

ChemistryAlkynylationTrifluoromethylCombinatorial chemistryOrganic chemistryCatalysisAlkylFluorine in Organic ChemistrySulfur-Based Synthesis TechniquesCarbohydrate Chemistry and Synthesis