Litcius/Paper detail

Electrochemical C–H Sulfonylation of Hydrazones

Biswajit Sarkar, Payel Ghosh, Alakananda Hajra

2023Organic Letters32 citationsDOI

Abstract

We have developed an electrochemical method for the direct C–H sulfonylation of aldehyde hydrazones using sodium sufinates as the sulfonylating agent under supporting electrolyte-free conditions. This straightforward sulfonylation strategy afforded a library of ( E )-sufonylated hydrazones with high tolerance of various functional groups. The radical pathway of this reaction has been revealed by the mechanistic studies.

Topics & Concepts

ChemistryElectrochemistryCombinatorial chemistryOrganic chemistryElectrodePhysical chemistrySulfur-Based Synthesis TechniquesRadical Photochemical ReactionsCatalytic C–H Functionalization Methods