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Chemical tuning of spin clock transitions in molecular monomers based on nuclear spin-free Ni(<scp>ii</scp>)

Marcos Rubín-Osanz, François Lambert, Feng Shao, Éric Rivière, Régis Guillot, Nicolas Suaud, Nathalie Guihéry, David Zueco, Anne‐Laure Barra, Talal Mallah, Fernando Luis

2021Chemical Science32 citationsDOIOpen Access PDF

Abstract

the modification of the ligand shell that determines the crystal field and the magnetic anisotropy. These properties are crucial to realize model spin qubits that combine the necessary resilience against decoherence, a proper interfacing with other qubits and with the control circuitry and the ability to initialize them by cooling.

Topics & Concepts

Quantum tunnellingSpin (aerodynamics)MonomerQuantum chemicalChemistryMoleculePhysicsMaterials scienceChemical physicsCondensed matter physicsNuclear magnetic resonanceQuantum mechanicsPolymerThermodynamicsMagnetism in coordination complexesOrganic and Molecular Conductors ResearchElectron Spin Resonance Studies
Chemical tuning of spin clock transitions in molecular monomers based on nuclear spin-free Ni(<scp>ii</scp>) | Litcius