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Metal-Free Regioselective N<sup>2</sup>-Arylation of 1<i>H</i>-Tetrazoles with Diaryliodonium Salts

Raktim Abha Saikia, Anurag Dutta, Bipul Sarma, Ashim Jyoti Thakur

2022The Journal of Organic Chemistry18 citationsDOI

Abstract

-tetrazoles with diaryliodonium salts to access 2-aryl-5-substituted-tetrazoles. Diaryliodonium salts with a wide range of both electron-rich and previously challenged electron-deficient aryl groups are applicable in this method. Diversely functionalized tetrazoles are tolerable also. We have devised a one-pot system to synthesize 2,5-diaryl-tetrazoles directly from nitriles. The synthetic utility of this method is furthered extended to late-stage arylation of two biologically active molecules.

Topics & Concepts

RegioselectivityChemistryArylCombinatorial chemistryMoleculeOrganic chemistryCatalysisAlkylSynthesis of Tetrazole DerivativesQuinazolinone synthesis and applicationsMulticomponent Synthesis of Heterocycles
Metal-Free Regioselective N<sup>2</sup>-Arylation of 1<i>H</i>-Tetrazoles with Diaryliodonium Salts | Litcius