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Towards effective indirect radioisotope energy converters with bright and radiation hard scintillators of (Gd,Y)3Al2Ga3O12 family

M. Korzhik, R. M. Αbashev, A. Fedorov, G. Dosovitskiy, E. Gordienko, I.A. Kamenskikh, D. Kazlou, D. Kuznecova, V. Mechinsky, В. А. Пустоваров, В. М. Ретивов, А. Н. Васильев

2022Nuclear Engineering and Technology21 citationsDOIOpen Access PDF

Abstract

Ceramics of quaternary garnets (Gd,Y)3Al2Ga3O12 doped with Ce, Tb have been fabricated and evaluated as prospective materials for indirect energy converters of α-and β-voltaic. Samples were characterized at excitation with an X-ray source and an intense 150 keV electron beam and showed good temperature stability of their emission and tolerance to irradiation. The role of X-rays accompanied the α-particle emitting in the increase of the conversion efficiency is clarified. The garnet-type structure of the matrix in the developed materials allows the production of quality crystalline mass with a light yield exceeding that of the commonly used YAG: Ce scintillator by a factor of two times.

Topics & Concepts

ScintillatorMaterials scienceCeramicRadiationIrradiationDopingYield (engineering)Cathode rayOptoelectronicsElectronOpticsNuclear physicsPhysicsMetallurgyDetectorRadiation Detection and Scintillator TechnologiesLuminescence Properties of Advanced MaterialsAdvanced Energy Technologies and Civil Engineering Innovations