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Giant orbital diamagnetism of three-dimensional Dirac electrons in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mrow><mml:msub><mml:mi>Sr</mml:mi><mml:mn>3</mml:mn></mml:msub><mml:mi>PbO</mml:mi></mml:mrow></mml:math> antiperovskite

S. Suetsugu, Kentaro Kitagawa, Toshikaze Kariyado, Andreas W. Rost, J. Nuss, Christiane Mühle, Masao Ogata, H. Takagi

2021Physical review. B./Physical review. B22 citationsDOIOpen Access PDF

Abstract

Interband mixing in Dirac semimetals has been known theoretically to give rise to a giant orbital diamagnetism when the Fermi level is close to the Dirac point. Here, the authors report a ${}^{207}$Pb NMR study on the three-dimensional Dirac antiperovskite system Sr${}_{3}$PbO. The analysis of the Knight shift, the magnetic susceptibility, and the spin-lattice relaxation rate for samples with different Fermi levels shows that the enhanced diamagnetism in the bulk magnetic susceptibility of Sr${}_{3}$PbO does indeed originate from the orbital contribution of Dirac electrons.

Topics & Concepts

DiamagnetismCondensed matter physicsPhysicsKnight shiftElectronMagnetic susceptibilitySuperconductivityQuantum mechanicsMagnetic fieldTopological Materials and PhenomenaGraphene research and applicationsThermal Expansion and Ionic Conductivity
Giant orbital diamagnetism of three-dimensional Dirac electrons in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mrow><mml:msub><mml:mi>Sr</mml:mi><mml:mn>3</mml:mn></mml:msub><mml:mi>PbO</mml:mi></mml:mrow></mml:math> antiperovskite | Litcius