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Expanding the functionality of proteins with genetically encoded dibenzo[<i>b</i>,<i>f</i>][1,4,5]thiadiazepine: a photo-transducer for photo-click decoration

Qin Xiong, Tingting Zheng, Xin Shen, Baolin Li, Jielin Fu, Xiaohu Zhao, Chunxia Wang, Zhipeng Yu

2022Chemical Science27 citationsDOIOpen Access PDF

Abstract

Via directed evolution of the tRNA synthetase, genetic encoding of a unique DBTD derived ncAA into proteins is realized. The DBTD residue is capable of transducing photon energy into ring-strain energy in situ for photo-clicking with diarylsydnone.

Topics & Concepts

TransducerClick chemistryComputational biologyComputer scienceChemistryBiologyCombinatorial chemistryEngineeringElectrical engineeringClick Chemistry and ApplicationsPhotochromic and Fluorescence ChemistryChemical Synthesis and Analysis
Expanding the functionality of proteins with genetically encoded dibenzo[<i>b</i>,<i>f</i>][1,4,5]thiadiazepine: a photo-transducer for photo-click decoration | Litcius