Recent Strategies for Ni3S2-Based Electrocatalysts with Enhanced Hydrogen Evolution Performance: A Tutorial Review
Yucheng Shen, Jixing Bai, Huijie Wei, Jun Gu, Qi Cao
Abstract
Water electrolysis represents one of the most environmentally friendly methods for hydrogen production, while its overall efficiency is primarily governed by the electrocatalyst. Nickel sulfides, e.g., Ni3S2, are considered to be highly promising catalysts for the hydrogen evolution reaction (HER) due to their distinctive chemical structure. However, the practical application of Ni3S2-based electrocatalysts is hindered by unsatisfactory high overpotential in the HER and weakened catalytic performance under alkaline conditions. Therefore, in this regard, further research on Ni3S2-based catalysts is being carried out to tackle these challenges. This review provides a comprehensive survey of the latest advancements in Ni3S2-based in improving the HER performance of Ni3S2-based electrocatalysts. The review may offer some inspiration for the rational design and synthesis of novel transition metal-based catalysts with enhanced water electrolysis performance.