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Self-Consistent Implementation of Kohn–Sham Adiabatic Connection Models with Improved Treatment of the Strong-Interaction Limit

Szymon Śmiga, Fabio Della Sala, Paola Gori‐Giorgi, Eduardo Fabiano

2022Journal of Chemical Theory and Computation22 citationsDOIOpen Access PDF

Abstract

dissociation, the SCF-ACM functionals yield significant improvements with respect to standard functionals also thanks to the use of the new GGAs for the strong-coupling functionals.

Topics & Concepts

Adiabatic processKohn–Sham equationsPerturbation theory (quantum mechanics)Hybrid functionalStatistical physicsDensity functional theoryPerturbation (astronomy)Atomic orbitalLimit (mathematics)PhysicsComputer scienceQuantum mechanicsMathematicsMathematical analysisElectronAdvanced Chemical Physics StudiesSpectroscopy and Quantum Chemical StudiesPerovskite Materials and Applications
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