Spatial separation of redox centers for boosting cooperative photocatalytic hydrogen evolution with oxidation coupling of benzylamine over Pt@UiO-66-NH<sub>2</sub>@ZnIn<sub>2</sub>S<sub>4</sub>
Lianlian Wang, Yujie Zhao, Bin Zhang, Gaigai Wu, Jie Wu, Hongwei Hou
Abstract
Pt@UiO-66-NH 2 @ZIS is prepared to realize the co-production of H 2 and C–N coupling products. DFT calculations of interfacial charges reveal that spatial separation of redox centers has a significant catalytic effect on dual-functional systems.
Topics & Concepts
RedoxCatalysisPhotocatalysisBoosting (machine learning)Hydrogen productionChemistryHydrogenBenzylaminePhotochemistryOxidative coupling of methaneMaterials scienceInorganic chemistryOrganic chemistryComputer scienceMachine learningAdvanced Photocatalysis TechniquesElectrocatalysts for Energy ConversionAdvanced Nanomaterials in Catalysis