Solvent-modulated second harmonic generation in <i>N</i> -alkylated thiohydantoin derivatives: synthesis, characterization, and first-principle insights
Muhammad Arif Ali, Muhammad Zahid Qureshi, Rahman Shah Zaib Saleem, Mariusz Mojzych, Ahsan Sharif, Muhammad Arshad
Abstract
= 8.8 ns for MAS3) further underscore the promise of these derivatives for optoelectronic applications. This work not only validates the solvent modulated EFISHG and EOPE capabilities of thiohydantoin-based systems but also provides a robust framework for designing advanced organic materials for photonics and telecommunications.
Topics & Concepts
HyperpolarizabilityMoleculeSecond-harmonic generationCharge (physics)Molecular orbitalBand gapChemistryElectric fieldComputational chemistryIntramolecular forceMolecular electronicsMolecular physicsHarmonicMaterials scienceOptoelectronicsDensity functional theoryNonlinear opticsChemical physicsFourier transform infrared spectroscopyVoltageField (mathematics)Solvent effectsInfraredWork (physics)High harmonic generationPhysical chemistrySpectroscopyRadiative transferPhotochemistry and Electron Transfer StudiesSpectroscopy and Quantum Chemical StudiesPhotonic and Optical Devices