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Chiral columns forming a lattice with a giant unit cell

Paulina Rybak, Adam Krówczyński, Jadwiga Szydłowska, Damian Pociecha, Ewa Górecka

2022Soft Matter12 citationsDOI

Abstract

lattice below the columnar hexagonal phase. The 3D columnar structure is a result of frustration imposed by the arrangement of helical columns of opposite chiralities into a triangular lattice. The studied materials exhibit fluorescence properties that could be easily tuned by modification of the molecular structure; for compounds with the extended π electron conjugated systems the fluorescence is quenched. For molecules with a flexible structure the fluorescence quantum yield reaches 25%. On the other hand, compounds with a more rigid mesogenic core, for which the fluorescence is suppressed, show effective photogeneration of charge carriers. For some materials bi-polar hole and electron transport was observed.

Topics & Concepts

MesogenColumnar phaseHexagonal latticeFluorescenceMaterials scienceCrystallographyLattice (music)Chemical physicsConjugated systemMoleculeLiquid crystalChemistryCondensed matter physicsMesophasePolymerLiquid crystallineOrganic chemistryOpticsOptoelectronicsPhysicsAntiferromagnetismComposite materialAcousticsLiquid Crystal Research AdvancementsPhotochemistry and Electron Transfer StudiesSynthesis and Properties of Aromatic Compounds
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