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Cross-Electrophile Coupling: Principles, Methods, and Applications in Synthesis

Lauren E. Ehehalt, Omar M. Beleh, Isabella C. Priest, Julianna M. Mouat, Alyssa K. Olszewski, Benjamin N. Ahern, Alexandro R. Cruz, K. Benjamin, Anthony J. Castro, Kai Kang, Jiang Wang, Daniel J. Weix

2024Chemical Reviews236 citationsDOIOpen Access PDF

Abstract

)-C(sp) bond formation. Additional chapters include alkene difunctionalization, alkyne difunctionalization, and formation of carbon-heteroatom bonds. Each chapter is generally organized with an initial summary of mechanisms followed by detailed figures and notes on methodological developments and ending with application notes in synthesis. While XEC is becoming an increasingly utilized approach in synthesis, its early stage of development means that optimal catalysts, ligands, additives, and reductants are still in flux. This review has collected data on these and various other aspects of the reactions to capture the state of the field. Finally, the data collected on the papers in this review is offered as Supporting Information for readers.

Topics & Concepts

ChemistryElectrophileCoupling (piping)Combinatorial chemistryComputational chemistryNanotechnologyBiochemical engineeringOrganic chemistryCatalysisMaterials scienceMechanical engineeringEngineeringChemical synthesis and alkaloidsAsymmetric Synthesis and CatalysisCatalytic Cross-Coupling Reactions