Litcius/Paper detail

Recent Progress of Single‐atom Catalysts in the Electrocatalytic Reduction of Oxygen to Hydrogen Peroxide

Weiya Zhu, Shaowei Chen

2020Electroanalysis39 citationsDOI

Abstract

Abstract Single‐atom catalysts (SACs) have been attracting extensive interest in the electrocatalytic production of hydrogen peroxide by oxygen reduction reaction (ORR). This is due to the maximal efficiency of atom utilization and intimate interaction of the metal centers with the supporting matrix that may be exploited for deliberate manipulation of the electrocatalytic activity and selectivity, in comparison with the conventional nanoparticle counterparts. Herein, we summarize recent progress of the design and engineering of SACs towards ORR for H 2 O 2 generation, based on both noble and non‐noble metals. We conclude the review with a perspective highlighting the promises and challenges involved in future research.

Topics & Concepts

Hydrogen peroxideCatalysisSelectivityCombinatorial chemistryNoble metalChemistryElectrocatalystOxygen atomOxygen reductionAtom (system on chip)HydrogenNanoparticleNanotechnologyOxygen reduction reactionMaterials scienceElectrochemistryElectrodeComputer scienceOrganic chemistryPhysical chemistryMoleculeEmbedded systemElectrocatalysts for Energy ConversionCatalytic Processes in Materials ScienceCO2 Reduction Techniques and Catalysts