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Ni single atoms supported on hierarchically porous carbonized wood with highly active Ni–N<sub>4</sub>sites as a self-supported electrode for superior CO<sub>2</sub>electroreduction

Huaiyu Chang, Hui Pan, Fang Wang, Zhengguo Zhang, Yaming Kang, Shixiong Min

2022Nanoscale34 citationsDOI

Abstract

A self-supported single-atom electrocatalyst was developed by anchoring Ni single atoms on porous N-doped carbonized wood (Ni SAs-NCW), showing a high performance in CO 2 electroreduction and potential to be integrated into the flow cell system.

Topics & Concepts

Materials scienceCarbonizationReversible hydrogen electrodeElectrolyteElectrodeChemical engineeringElectrolysisNanotechnologyPorosityCarbon fibersElectrocatalystFaraday efficiencyCatalysisComposite materialWorking electrodeElectrochemistryChemistryPhysical chemistryComposite numberOrganic chemistryScanning electron microscopeEngineeringCO2 Reduction Techniques and CatalystsIonic liquids properties and applicationsElectrocatalysts for Energy Conversion
Ni single atoms supported on hierarchically porous carbonized wood with highly active Ni–N<sub>4</sub>sites as a self-supported electrode for superior CO<sub>2</sub>electroreduction | Litcius