Litcius/Paper detail

Three-Component Electrochemical Aminoselenation of 1,3-Dienes

Sai-Yan Ren, Qi Zhou, He‐Yang Zhou, Lin‐Wei Wang, Olga M. Mulina, Stanislav A. Paveliev, Haitao Tang, Alexander O. Terent’ev, Ying‐Ming Pan, Xiu‐Jin Meng

2023The Journal of Organic Chemistry27 citationsDOI

Abstract

Azoles and organoselenium compounds are pharmacologically important scaffolds in medicinal chemistry and natural products. We developed an efficient regioselective electrochemical aminoselenation reaction of 1,3-dienes, azoles, and diselenide derivatives to access selenium-containing allylazoles skeletons. This protocol is more economical and environmentally friendly and features a broad substrate scope; pyrazole, triazole, and tetrazolium were all tolerated under the standard conditions, which could be applied to the expedient synthesis of bioactive molecules and in the pharmaceutical industry.

Topics & Concepts

DiselenideRegioselectivityChemistryPyrazoleCombinatorial chemistryEnvironmentally friendlySubstrate (aquarium)ElectrochemistryOrganic chemistryAntifungalSeleniumCatalysisElectrodeOceanographyPhysical chemistryBiologyMedicineDermatologyEcologyGeologySulfur-Based Synthesis TechniquesOrganoselenium and organotellurium chemistryRadical Photochemical Reactions