Litcius/Paper detail

Double-Confined Ultrafine Cobalt Clusters for Efficient Peroxide Activation

Xiaowen Xie, Mingshan Zhu, Fei Xiao, Yongjie Xiang, Huanran Zhong, Zhimin Ao, Haibao Huang

2023JACS Au20 citationsDOIOpen Access PDF

Abstract

High Resolution Image Download MS PowerPoint Slide The construction of highly active catalysts presents great prospects, while it is a challenge for peroxide activation in advanced oxidation processes (AOPs). Herein, we facilely developed ultrafine Co clusters confined in mesoporous silica nanospheres containing N-doped carbon (NC) dots (termed as Co/ [email protected] 2 ) via a double-confinement strategy. Compared with the unconfined counterpart, Co/ [email protected] 2 exhibited unprecedented catalytic activity and durability for removal of various organic pollutants even in extremely acidic and alkaline environments (pH from 2 to 11) with very low Co ion leaching. Experiments and density functional theory (DFT) calculations proved that Co/ [email protected] 2 possessed strong peroxymonosulphate (PMS) adsorption and charge transfer capability, enabling the efficient O–O bond dissociation of PMS to HO • and SO 4 •– radicals. The strong interaction between Co clusters and mSiO 2 containing NC dots contributed to excellent pollutant degradation performances by optimizing the electronic structures of Co clusters. This work represents a fundamental breakthrough in the design and understanding of the double-confined catalysts for peroxide activation.

Topics & Concepts

CatalysisPeroxideDissociation (chemistry)CobaltAdsorptionMesoporous silicaLeaching (pedology)Mesoporous materialChemistryChemical engineeringPollutantDensity functional theoryMaterials sciencePhotochemistryNanotechnologyInorganic chemistryPhysical chemistryOrganic chemistryComputational chemistrySoil scienceEngineeringSoil waterEnvironmental scienceAdvanced Photocatalysis TechniquesCatalytic Processes in Materials ScienceAdvanced Nanomaterials in Catalysis